Publication Details

Category Text Publication
Reference Category Journals
DOI 10.1016/j.watres.2023.119861
Title (Primary) Is adsorption onto activated carbon a feasible drinking water treatment option for persistent and mobile substances?
Author Schumann, P.; Muschket, M.; Dittmann, D.; Rabe, L.; Reemtsma, T.; Jekel, M.; Ruhl, A.S.
Source Titel Water Research
Year 2023
Department ANA
Volume 235
Page From art. 119861
Language englisch
Topic T9 Healthy Planet
Abstract Persistent and mobile (PM) substances among the organic micropollutants have gained increasing interest since their inherent properties enable them to enrich in water cycles. This study set out to investigate the potential of adsorption onto activated carbon as a drinking water treatment option for 19 PM candidates in batch experiments in a drinking water matrix using a microporous and a mesoporous activated carbon. Overall, adsorption of PM candidates proved to be very variable and the extent of removal could not be directly related to molecular properties. At an activated carbon dose of 10 mg/L and 48 h contact time, five (out of 19) substances were readily removed (≥ 80%), among them N-(3-(dimethylamino)-propyl)methacrylamide, which was investigated for the first time. For five other substances, no or negligible removal (< 20%) was observed, including 2-methyl-2-propene-1-sulfonic acid and 4‑hydroxy-1-(2-hydroxyethyl)-2,2,6,6,-tetramethylpiperidine. For the former, current state of the art adsorption processes may pose a sufficient barrier. Additionally, substance specific surrogate correlations between removals and UVA254 abatements were established to provide a cheap and fast estimate for PM candidate elimination. Adsorption onto activated carbon could contribute significantly to PM substance elimination as part of multi barrier approaches, but assessments for individual substances still require clarification, as demonstrated for the investigated PM candidates.
Persistent UFZ Identifier https://www.ufz.de/index.php?en=20939&ufzPublicationIdentifier=23368
Schumann, P., Muschket, M., Dittmann, D., Rabe, L., Reemtsma, T., Jekel, M., Ruhl, A.S. (2023):
Is adsorption onto activated carbon a feasible drinking water treatment option for persistent and mobile substances?
Water Res. 235 , art. 119861 10.1016/j.watres.2023.119861