Details zur Publikation

Kategorie Textpublikation
Referenztyp Zeitschriften
DOI 10.1021/acs.estlett.4c00866
Lizenz creative commons licence
Titel (primär) Effect-based water quality assessment in an urban tributary under base flow and storm conditions
Autor Rauert, C.; König, M.; Neale, P.A.; Thomas, K.V.; Escher, B.I. ORCID logo
Quelle Environmental Science & Technology Letters
Erscheinungsjahr 2024
Department ZELLTOX
Band/Volume 11
Heft 12
Seite von 1314
Seite bis 1320
Sprache englisch
Topic T9 Healthy Planet
Supplements https://ndownloader.figstatic.com/files/50791652
https://ndownloader.figstatic.com/files/50791655
Keywords bioassays; effect-based trigger value; neurotoxicity; stormwater; tire additive chemicals
Abstract Storm events can mobilize organic contaminants from hard surfaces in urban areas and can impact receiving water quality. Traditional water quality assessments predominantly rely on chemical analysis, which inadequately capture the collective effects of diverse chemical mixtures released during storm events. We applied effect-based methods (EBM) to detect arylhydrocarbon receptor (AhR) activity, estrogenic activity, neurotoxicity and oxidative stress response in water samples from an urban tributary during a storm event and compared it with base flow conditions. AhR activity and neurotoxicity peaked during the storm event, with neurotoxicity exceeding the interim effect-based trigger value and showing a high specificity of effect. This suggests unacceptable water quality during the storm event. Conversely, estrogenic activity was relatively low, and there was little difference between base flow conditions and the storm event. The absence of wastewater, industrial and agricultural inputs in the catchment suggests that the observed bioactivity was related to road runoff, specifically from two adjacent major motorways. The effects on AhR and neurotoxicity were linearly correlated with detected concentrations of 15 tire additive chemicals from an accompanying study. This study demonstrates that EBM provides complementary information to chemical analysis for water quality monitoring and that there is an increased chemical pressure on receiving water bodies during rain events in urban areas.
dauerhafte UFZ-Verlinkung https://www.ufz.de/index.php?en=20939&ufzPublicationIdentifier=29941
Rauert, C., König, M., Neale, P.A., Thomas, K.V., Escher, B.I. (2024):
Effect-based water quality assessment in an urban tributary under base flow and storm conditions
Environ. Sci. Technol. Lett. 11 (12), 1314 - 1320 10.1021/acs.estlett.4c00866