Details zur Publikation

Kategorie Textpublikation
Referenztyp Zeitschriften
DOI 10.1080/10256010701360132
Titel (primär) Anomalous fluoride concentration in groundwater - is it natural or pollution? A stable isotope approach
Autor Marimon, M.P.C.; Knöller, K.; Roisenberg, A.
Quelle Isotopes in Environmental and Health Studies
Erscheinungsjahr 2007
Department ISOHYD
Band/Volume 43
Heft 2
Seite von 165
Seite bis 175
Sprache englisch
Keywords Fertiliser contamination; Fluoride; Groundwater; Hydrogen-2; Nitrogen-15; Oxygen-18; Sulphur-34
Abstract Fluoride anomalies (up to 11 mg/l) have been detected in groundwater of the central region of Rio Grande do Sul State, Southern Brazil, in an area where fluorosis is endemic. Two hypotheses are investigated concerning the fluoride origin: lithochemical affiliation from regional rock or contamination by fertilisers application. These hypotheses are discussed based on the stable isotope data of water, nitrate, and sulphate, which indicates that the local precipitation is the main groundwater recharge source. The isotopic composition of groundwater sulphate is similar to that of fertiliser sulphate. However, a conclusive assignment of groundwater sulphate to fertiliser origin is not indicated because further possible sulphate sources fall into the same isotopic range. In contrast, the isotopic composition of dissolved nitrate suggests that there is no direct relationship to the use of NPK fertilisers. Hence, an origin of the high fluoride content in groundwater related to long-term rock-water interactions seems likely.
dauerhafte UFZ-Verlinkung https://www.ufz.de/index.php?en=20939&ufzPublicationIdentifier=2043
Marimon, M.P.C., Knöller, K., Roisenberg, A. (2007):
Anomalous fluoride concentration in groundwater - is it natural or pollution? A stable isotope approach
Isot. Environ. Health Stud. 43 (2), 165 - 175 10.1080/10256010701360132